Abstract
SynopsisThree body fragmentation pathways of OCS3+ molecular ion leading to detection of C+ + O+ + S+ in coincidence have been studied using the technique of recoil ion momentum spectroscopy. This fragmentation can occur either via a one step concerted process or a two step sequential process. In the first step of the sequential pathway either CO2+ or CS2+ is formed. By separating the events coming from the two processes, branching ratios are determined and the possible electronic states associated with the intermediate CO2+ or CS2+ have been identified.
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