Abstract
Observed vibration—rotation constants for HCO/DCO and HO 2/DO 2 are combined with vibrational frequencies and ground-state rotational constants in order to derive harmonic as well as third-order anharmonic potential constants, and also equilibrium structure parameters for the formyl and hydroperoxyl radicals. The “diagonal” terms of the third-order anharmonic constants thus obtained for the stretching modes are discussed in terms of the diatomic-molecule model.
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