Abstract
A numerical investigation is made of third harmonic generation (THG) under conditions of two-photon resonance between the fundamental frequency and a selected transition in the atoms of a medium. It is shown that under conditions of coherent interaction between the pump pulse and the medium, a THG efficiency of ~20% or higher may be achieved. In this case, THG in the form of high-power ultrashort pulses may be obtained. It is shown that experimental observation of similar effects in specific media should not present particular difficulties.
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