Abstract

Interest in developing advanced flexible materials that are stable, mechanically deformable, lightweight, cost-effective, and eco-friendly is ever-growing to support high-performance state-of-the-art wearable electronic devices. Another critical requirement of wearable devices is low energy consumption during operation for prolonged use. Herein, we demonstrate a compressible electrochromic device (ECD) using the three-dimensional (3D) compressible sponge electrolyte layer. A 3D porous sponge was fabricated using a facile and eco-friendly method of leaching sugar, a pore-creating agent, from an UV-cured skeletal structure. The simple structure of a compressible ECD is advantageous for its applicability as an optical tactile sensor device. A low-voltage operation, as evidenced by optical measurements, can ensure the long-term performance of the sensor. Furthermore, the color change in the ECD that occurs with the applied pressure acts as an effective pressure-sensing mechanism for the system involved. Thus, compressible sponge electrolytes layers are promising for various wearable tactile device applications.

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