Abstract
Values of G E, H E, and V E for cycloalkane + 2,3-dimethylbutane mixtures have been calculated from various equations of state and the results compared with experiment. The predictions of the van der Waals type equations of state are superior to those of a corresponding states treatment based on an empirical equation of state for the “simple” fluids. Further, the van der Waals type equations are more successful when the pure-fluid parameters are adjusted to fit the properties of the liquid rather than the gas-liquid critical constants. Overall the theory proposed by Flory gives the best results.
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