Abstract
According to measured experimental phase diagram data and thermodynamic data, the HoCl3-MCl (M = Na, K, Rb, Cs) phase diagrams were determined by the CALPHAD technique. The Gibbs energies of liquid phases in these systems have been optimized and calculated by the modified quasi-chemical model in the pair-approximation for short-range ordering. A series of thermodynamic functions have been optimized and calculated on the basis of an interactive computer-assisted analysis. The results show that the thermodynamic properties and phase diagrams are self-consistent. The optimized results for the systems are discussed.
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