Abstract

We analyze in this paper the process of double-electron ejection through two-photon absorption from the fundamental state of helium. We focus on the case of photon energies close to 2 a.u., which marks the threshold between direct and sequential double-ionization regimes. We demonstrate the crucial role of two-photon excitation-plus-ionization process of ${\mathit{nlk}}^{\ensuremath{'}}{l}^{\ensuremath{'}}$ Rydberg series. We show that the latter channel must be taken into account in the theory in order to properly describe two-electron ejection. A simple expression is derived for the electron energy spectrum, leading to better insights into the physics underlying two-photon absorption close to the sequential threshold.

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