Theoretical study of anisotropy-induced extrinsic chirality and chiral discrimination of surface plasmon polaritons

Abstract

We present the characteristics of a simple waveguiding structure constructed by anisotropic birefringent crystal-metal-chiral medium, anisotropic-metal-chiral in short, and reveal the chiral-dependent dispersion and propagation properties of the surface plasmon polaritons (SPPs). We demonstrate its remarkable discrimination ability to the magnitude and sign of both the real and imaginary part of the chirality parameter. The anisotropy plays a key role in such performance and shows tuneable ability in enantiomeric discrimination even when the chirality parameter is complex-valued. Most importantly, the physical origin of chiral discrimination stems from the extrinsic chirality of the system, which arises from the mutual orientation of the SPPs and the optical axis. Moreover, we also clarify the fundamental physics behind the chiral discriminating behaviour by associating the intrinsic quantum spin Hall effect (QSHE) of the SPPs with the electromagnetic field analysis. This structure does not rely on complicated fabrication but provides the opportunity of on-chip surface-sensitive biosensing. We anticipate that our work will stimulate intensive research to investigate the anisotropy-induced chiral sensing techniques in plasmonic platforms.