Abstract

The temperature dependence of the domain structure of single crystals of uniaxial ferrimagnetic oxides with high-anisotropy field in the SrO( <tex xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink">6 - x</tex> )Fe <inf xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink">2</inf> O <inf xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink">3</inf> <tex xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink">x</tex> Al <inf xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink">2</inf> O <inf xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink">3</inf> compositional series, with <tex xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink">x = 1.8</tex> and 2.4, was investigated. The domain configurations of thermally and/or ac field demagnetized states and the changes in dc and ac fields were observed by means of the colloid technique using a suspension in paraffine oil. The temperature dependence of the wall energy density between room temperature and the Curie point (270°C) of the compound with <tex xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink">x = 1.8</tex> was computed using the temperature dependence of the saturation magnetization and the domain width for the Kittel-like domain structure. It has been found that the room temperature domain structure of the compound with <tex xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink">x = 2.4</tex> depends upon the mode of demagnetization, i.e., thermally or in the ac field. The ac demagnetized states are more stable than the thermally demagnetized ones. The samples exhibit a room temperature memory of the previous magnetization, which decreases with rising temperature. This memory is completely lost after heating at 400°C. The peculiarities of the temperature dependence of the domain structure and magnetic behavior on thermal cycling are explained by considering the existence of magnetic inhomogeneities within the crystal.

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