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Abstract
The deprotonated derivative pyridine-2-thiolato (PyS~-) of pyridine-2-thione (PySH)is a potentially amibidentate or multi-functional donor which coordinates toward transitionmetals with either the exocyclic S or heterocyclic N atom or both atoms to form differentcoordination modes. We have recently reported the synthesis and crystal structure ofthe first dinuclear molybdenum complex with doubly-bridging PyS ligands [Mo_2(CO)_4(μ-PyS)_2(PPh_3)_2]which was obtained from the reaction of [Mo(CO)_3(CH_3CN)_3] with
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