Abstract
A systematic study of the crystal structures of (BEDT-TTF) 2X salts [BEDT-TTF is bis-(ethylenedithio) tetrathiafulvalene, C 10S 8H 8, and X is a linear trihalide anion] reveal that the different packing motifs for the BEDT-TTF molecules are directly related to the electrical properties of these materials. The packing of the organic molecules is influenced by the cation-anion interactions of the -CH 2…X − type and is observed to change systematically with anion size.
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