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Abstract
Abstract The γ-ray-induced oxidation of toluene in liquid carbon dioxide has been reinvestigated. In order to discuss the precursors of the main products: three kinds of cresols and benzyl alcohol, 1-butene was used as the scavenger of oxygen atoms. The formation of cresols and benzyl alcohol was well explained by the participation of two precursors: one is oxygen atoms and the other is ionic species, O− or/and CO3− ions. The ratio of the G-value of oxygen atoms to that of the sum of O− and CO3− ions initially formed was estimated to be 4 : 1 for pure liquid carbon dioxide. The spur model previously proposed was applied to explain the formation of O− and CO3− ions.
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