Abstract
AbstractMagneto‐structural correlations in Cu(en )2Pt(CN)4 (en = C2H8N2) have been investigated by experimental studies of the magnetic properties and hydrogen bond geometry. The analysis of electron paramagnetic resonance spectra confirmed the d z2 electronic ground state of Cu(II) ion expected from room temperature X‐ray measurements. Magnetization and susceptibility data indicate the presence of weak exchange coupling J /k B = –0.4 K. Consequently, a spin diffusive regime in the spin relaxation can be expected at 4 K, and the angular dependence of the linewidth can be qualitatively explained by considering two‐dimensional magnetic behaviour. (© 2006 WILEY‐VCH Verlag GmbH & Co. KGaA, Weinheim)
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