Abstract

Monte Carlo simulation data from the two-dimensional facilitated kinetic Ising model proposed by Fredrickson and Andersen is examined with the goal of understanding the processes responsible for the characteristic features of glassy dynamics. The spatial distribution of spin flip rates is found to be highly nonuniform with pockets of rapidly relaxing spins surrounded by kinetically locked domains. The slow relaxation of these latter domains, which gives rise to the characteristic long time tail of the linear response function, is due to the action of rare clusters of spins which are able to propagate their influence throughout the sample. An analytic expression is derived for the density of these active sites which is found to fully account for the non-Arrhenius temperature dependence of the relaxation time in this model. The consequences of these results for both theories and experiments in structural glasses are discussed.

Full Text
Paper version not known

Talk to us

Join us for a 30 min session where you can share your feedback and ask us any queries you have

Schedule a call

Disclaimer: All third-party content on this website/platform is and will remain the property of their respective owners and is provided on "as is" basis without any warranties, express or implied. Use of third-party content does not indicate any affiliation, sponsorship with or endorsement by them. Any references to third-party content is to identify the corresponding services and shall be considered fair use under The CopyrightLaw.