The Non-Monotonic Response of Cumulus Congestus to the Concentration of Cloud Condensation Nuclei

Abstract

This study uses idealized simulations to investigate the impact of cloud condensation nuclei (CCN) on a cumulus congestus. Thirteen cases with the initial CCN_C, which is the CCN concentration at 1% supersaturation with respect to water, from 10 to 10,000 cm−3 are simulated. The analysis focuses on the liquid phase due to the negligible ice phase in this study. A non-monotonic response of cloud properties and precipitation to CCN concentration is observed. When CCN_C is increased from 10 to 50 cm−3, the enhanced condensation due to the more numerous droplets invigorates the cumulus congestus. The delayed precipitation formation due to the smaller droplets also facilitates the cloud development. The two processes together lead to a higher liquid water path (LWP), higher cloud top, and heavier precipitation. The cumulus congestus has the highest cloud top, the strongest updraft, and the most accumulated precipitation and at CCN_C = 50 cm−3. When CCN_C is increased from 50 to 500 cm−3, the condensation near the cloud base is further enhanced and the precipitation is further delayed, both of which lead to more liquid water remaining in the cloud, and thus an even higher LWP and heavier precipitation rate in the later stage. However, the significantly enhanced evaporation near the cloud top limits the vertical development of the cumulus congestus, leading to a lower cloud top. When CCN_C is further increased to be higher than 1000 cm−3, the cumulus congestus is strongly suppressed, and no precipitation forms. The ratio of the precipitation production rate to vertical cloud water flux in the updraft is not a constant, as is generally assumed in cumulus parameterization schemes, but decreases significantly with increasing CCN concentration. It is also found that the CCN effect on the cumulus congestus relies on which parameters are used to describe the cloud strength. In this study, as CCN_C increases, the LWP and the maximum precipitation rate peak at CCN_C = 500 cm−3, while the cloud top height, maximum updraft, and accumulated precipitation amount peak at CCN_C = 50 cm−3.