Abstract
Ab initio calculations at the MP2 level and gas electron-diffraction data of (CH 3) 2TeCl 2 show that the molecular structure is pseudo-trigonal bipyramidal with the two methyl groups occupying equatorial positions and the two Cl atoms axial positions. The bond distances are ( GED MP2 ): TeC = 213.2(5)/214.6 pm, TeCl = 250.4(3)/261.8 pm and the valence angles ∠ CTeC = 97(5)° 97.6° ; ∠ ClTeCl = 170(2)° 170.8° .
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