Abstract

Magnetic neutron diffraction measurements have been performed on (Co 1− x Mg x )O solid solutions with x = 0.1, 0.2, 0.3, 0.43, 0.53, 0.63 and 0.7 at T = 4.2 –300 K. It is shown that the concentration dependence of the average magnetic moment per atom does not obey the condition of simple dilution. The diamagnetic atom results in a local canting of the moments and an additional reduction of the average magnetic moment. One can consider this atom as a source of random magnetic field due to the appearance of a new superexchange interaction between magnetic atoms through the diamagnetic impurity. The sign of this interaction is opposite to the sign of the direct exchange interaction in the magnetic sublattice.

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