Abstract
Using two Ge detectors, the high-resolution Doppler-broadening energy spectra of positron annihilation gamma rays has been obtained by measuring the coincidences of the two photons. Light bleaching and oxygen effects on positron annihilation were investigated in this way. A large enhancement of the high-momentum part of the coincidence Doppler spectra was observed in poly(methylmethacrylate) (PMMA), which contains oxygen atoms in the polymer structure. Bleaching experiments in PMMA and in copolymer ethylene-methylmethacrylate EMMA (LDPE+MMA 3 mol%) have demonstrated that the enhancement effect may be due to the trapping of positrons by the polar C +O − groups, followed by positron annihilation with the electrons belonging to oxygen.
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