Abstract

This paper demonstrates the role of meteorology and air transport in influencing the South African atmospheric CO2 distribution. CO2 data from December 2004 to December 2009 acquired by the Tropospheric Emission Spectrometer (TES) instrument onboard the Aura satellite were used to establish the CO2 vertical distribution at selected regions in South Africa. The Hybrid Single-Particle Lagrangian Integrated Trajectories (HYSPLIT) atmospheric model backward trajectories were used to determine the long-range air transport impacting on South African CO2 atmospheric distribution and to detect the source areas of air masses impacting on South Africa’s atmosphere. The study found that long-range air transport can result in the accumulation or dilution of atmospheric CO2 at various sites in South Africa, depending on the source region and type of air flow. The long-range air transport from different source regions at the upper air level between the 700 and 500 hPa stable layers and the layer above 500 hPa strengthens the inhomogeneity in the vertical distribution of CO2, which is caused by the decoupling effect of the upper air stable layers. This long-range air transport also involves intercontinental air transport.

Highlights

  • Free troposphere and stratospheric CO2 is a long-lived greenhouse gas (LLGHG), which is an effective tracer of atmospheric dynamics and transport in these layers

  • This study demonstrated that the relative atmospheric loading of CO2 at various regions in South

  • Meteorology and air transport play an important role in influencing the atmospheric mixing ratio distribution of CO2 in

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Summary

Introduction

Free troposphere and stratospheric CO2 is a long-lived greenhouse gas (LLGHG), which is an effective tracer of atmospheric dynamics and transport in these layers. It has an atmospheric lifetime of 50 to 200 years [1,2] and contributes about 66% of the gaseous radiative forcing responsible for anthropogenic climate change. Among the LLGHGs, CO2 increases have caused the largest sustained radiative forcing over the past decade [1,3,4,5,6,7,8,9]. Other sources include emissions due to land use changes such as deforestation and biomass burning [1,3,4,7,8,9,10,11]

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