Abstract
In a double saturation spectroscopy experiment, using the radiation from one single frequency cw laser, the spectra of 129I2 and 127I129I from one saturation setup were recorded simultaneously and with respect to the spectrum of 127I2 from another setup while tuning the laser. The hyperfine patterns of 129I2 and 127I129I were analysed to determine the nuclear electric quadrupole interaction and the nuclear spin–rotation interaction parameters. Models are presented describing the observations and giving reliable predictions for the hyperfine parameters of all isotopomers.
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