Abstract
The dissociation of the ions COCl 2 + and COF 2 + has been studied by photoelectron—photoion coincidence techniques over wide ranges of initial ion internal energies. Breakdown diagrams have been derived and the energy released into translation computed from the time-of-flight peak contours. The average kinetic energy releases are much greater than statistical predictions, especially at low parent internal energies, and the energy distributions do not, in general, agree with those calculated from the Klots model. Possible explanations for these differences are discussed.
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