Abstract

A large amount of volcanic ash produced during explosive volcanic eruptions has been found to sediment as aggregates of various types that typically reduce the associated residence time in the atmosphere (i.e., premature sedimentation). Nonetheless, speculations exist in the literature that aggregation has the potential to also delay particle sedimentation (rafting effect) even though it has been considered unlikely so far. Here, we present the first theoretical description of rafting that demonstrates how delayed sedimentation may not only occur but is probably more common than previously thought. The fate of volcanic ash is here quantified for all kind of observed aggregates. As an application to the case study of the 2010 eruption of Eyjafjallajökull volcano (Iceland), we also show how rafting can theoretically increase the travel distances of particles between 138–710 μm. These findings have fundamental implications for hazard assessment of volcanic ash dispersal as well as for weather modeling.

Highlights

  • A large amount of volcanic ash produced during explosive volcanic eruptions has been found to sediment as aggregates of various types that typically reduce the associated residence time in the atmosphere

  • Sedimentation of volcanic ash needs to be accurately described both for real-time forecasting of atmospheric dispersal and long-term hazard assessment of ground tephra loading in order to reduce risk associated with explosive volcanic eruptions[1,2]

  • We explore here how aggregation may not always reduce the residence time of volcanic ash in the atmosphere but, in some cases, may raft coarse ash acting as aggregate cores to larger distances from the volcano than expected (Fig. 1)

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Summary

Introduction

A large amount of volcanic ash produced during explosive volcanic eruptions has been found to sediment as aggregates of various types that typically reduce the associated residence time in the atmosphere (i.e., premature sedimentation). We demonstrate that rafting may occur under specific conditions due to the non-linear behavior between weight and drag forces acting on aggregates when falling through the atmosphere This information is summarized in dedicated sedimentation charts (described in section 2.1), a powerful tool to investigate the fate of volcanic ash in the atmosphere. A specific packing configuration (i.e., aggregate porosity φA and aggregate-to-core size ratio Λ) is required to trigger particle rafting Under this condition, the concurrent presence of fine and coarse ash in a given aggregate has the potential to simultaneously reduce the residence time of fine ash in the atmosphere and increase the sedimentation distance of coarse ash. The main objective of this paper is to identify the theoretical boundaries under which premature or delayed sedimentation of volcanic ash occurs during tephra fallout and how this affects the transport of volcanic ash in the atmosphere

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