Abstract

Abstract. Colluvial soils are enriched in soil organic carbon (SOC) in comparison to the soils of upslope areas due to the deposition and progressive burial of SOC. This burial of SOC has important implications for the global carbon cycle, but the long-term dynamics of buried SOC remain poorly constrained. We addressed this issue by determining the SOC burial efficiency (i.e. the fraction of originally deposited SOC that is preserved in colluvial deposits) of buried SOC as well as the SOC stability in colluvial soils. We quantified the turnover rate of deposited SOC by establishing sediment and SOC burial chronologies. The SOC stability was derived from soil incubation experiments and the δ13C values of SOC. The C burial efficiency was found to decrease with time, reaching a constant ratio of approximately 17% by about 1000–1500 yr post-burial. This decrease is attributed to the increasing recalcitrance of the remaining buried SOC with time and a less favourable environment for SOC decomposition with increasing depth. Buried SOC in colluvial profiles was found to be more stable and degraded in comparison to SOC sampled at the same depth at a stable reference location. This is due to the preferential mineralisation of the labile fraction of the deposited SOC. Our study shows that SOC responds to burial over a centennial timescale; however, more insight into the factors controlling this response is required to fully understand how this timescale may vary, depending on specific conditions such as climate and depositional environment.

Highlights

  • There are significant uncertainties associated with our understanding of the role of soil erosion in the global C cycle (e.g. Van Oost et al, 2007; Berhe et al, 2007; Lal, 2003)

  • These uncertainties originate from the difficulties associated with quantifying the fate of the eroded soil organic carbon (SOC)

  • The study area has a long history of agricultural land use: deciduous forests covered the catchment during the first half of the Holocene and the first agricultural crops appeared 4000–5000 yr ago

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Summary

Introduction

There are significant uncertainties associated with our understanding of the role of soil erosion in the global C cycle (e.g. Van Oost et al, 2007; Berhe et al, 2007; Lal, 2003). These uncertainties originate from the difficulties associated with quantifying the fate of the eroded soil organic carbon (SOC). Rather than reaching the fluvial system, where previously eroded SOC can be stored effectively in freshwater sediments, a substantial fraction of the sediment mobilised by soil erosion is re-deposited within the landscape in colluvial stores. The hillslope sediment delivery ratio, i.e. the ratio between the amount of sediment mobilised by erosion and exported to the fluvial system, for agricultural catchments in temperate climates is estimated to be between 20 and 50 % (Rommens et al, 2005; Notebaert et al, 2011; Trimble, 1999; Wang et al, 2010). 50–80 % of the eroded sediments are re-deposited on hillslopes and form colluvial soils (Wang et al, 2010)

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