Abstract
The far-infrared spectrum of nitryl chloride was studied using high-resolution Fourier-transform spectroscopy in the 300–525 cm−1region. Vibrational band centers of fundamental, hot, and difference bands were determined. Furthermore, rotational and centrifugal distortion constants up to fourth order for the ν3bands of35ClNO2and37ClNO2(centered at 370 and 364 cm−1, respectively) were obtained. The ν5fundamental of ClNO2(predicted around 410 cm−1) is very weak and overlapped by difference bands.
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