Abstract
Abstract Elements of the tensors of molecular polarizability changes in the single vibrations (the α′-elements) may be obtained from single crystal Raman work if the “oriented gas hypothesis” is applicable. From work on phosphonitrilic halides, relations between some of the α′ in the normal vibrations of triatomic groups have been extracted. Certain relations derived for p-chloroaniline are in accord with calculated values for benzene, but they require new concepts about the forms of the normal vibrations connected with the substituents. The apparent absence of interpretations of the α′ in most single crystal work is regretted.
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