Abstract
Abstract The hybrid donor between bis(ethylenedithio)tetrathiafulvalene and -tetraselenafulvalene (ET and BETS, respectively) has been synthesized and the electrical properties together with the crystal structures of its cation radical salts investigated. All of the crystals studied by X-ray structural analysis turned out to have an orientational disorder at the donor site. Although some of the charge-transfer salts were found to be isostructural with the corresponding ET and/or BETS salts, not all of their electrical properties are parallel to them; some are similar, others are significantly different from those of the parent donor salts. Such a trend indicates that the effect of the disorder on the electrical behavior might not be always equal, and should depend on some factor(s) yet to be clarified.
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