Abstract

La1−xSrxCoO3 (x = 0.18, 0.33, and 0.5) films were grown epitaxially on piezoelectric Pb(Mg1/3Nb2/3)O3-PbTiO3 substrates by pulsed laser deposition. The magnetization of these films varies with the external electric field, showing the magnetoelectric effect. With different doping content of Sr2+ ions, the change of magnetization for these films show different behaviors with increasing temperature, which can be attributed to the competition between electric-field-induced changes of spin state and double exchange interaction. This work presents an alternative mechanism to investigate the electric field control of magnetism in magnetoelectric heterostructure by tuning the spin state.

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