Abstract

Abstract. We present a description and evaluation of the Chemistry-Climate Model (CCM) LMDz-REPROBUS, which couples interactively the extended version of the Laboratoire de Météorologie Dynamique General Circulation Model (LMDz GCM) and the stratospheric chemistry module of the REactive Processes Ruling the Ozone BUdget in the Stratosphere (REPROBUS) model. The transient simulation evaluated here covers the period 1980–1999. The introduction of an interactive stratospheric chemistry module improves the model dynamical climatology, with a substantial reduction of the temperature biases in the lower tropical stratosphere. However, at high latitudes in the Southern Hemisphere, a negative temperature bias, that is already present in the GCM version, albeit with a smaller magnitude, leads to an overestimation of the ozone depletion and its vertical extent in the CCM. This in turn contributes to maintain low polar temperatures in the vortex, delay the break-up of the vortex and the recovery of polar ozone. The latitudinal and vertical variation of the mean age of air compares favourable with estimates derived from long-lived species measurements, though the model mean age of air is 1–3 years too young in the middle stratosphere. The model also reproduces the observed "tape recorder" in tropical total hydrogen (=H2O+2×CH4), but its propagation is about 30% too fast and its signal fades away slightly too quickly. The analysis of the global distributions of CH4 and N2O suggests that the subtropical transport barriers are correctly represented in the simulation. LMDz-REPROBUS also reproduces fairly well most of the spatial and seasonal variations of the stratospheric chemical species, in particular ozone. However, because of the Antarctic cold bias, large discrepancies are found for most species at high latitudes in the Southern Hemisphere during the spring and early summer. In the Northern Hemisphere, polar ozone depletion and its variability are underestimated in the simulation.

Highlights

  • Climate change and stratospheric ozone are coupled issues (World Meteorological Organisation/United Nations Environment Program (WMO/UNEP), 2007)

  • (mat tihdedsulme)mearntimdetphoelairrstdraitoffpeaursee.nces shown in stepsaowfar5m bKia.s at the tropical tropopause, which is a clear indication that this bias in General Circulation Model (GCM) was probably due to the specifi

  • We have developed the LMDz-REPROBUS chemistryclimate model, which couples interactively a general circulation model and a stratospheric chemistry module

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Summary

Introduction

Climate change and stratospheric ozone are coupled issues (World Meteorological Organisation/United Nations Environment Program (WMO/UNEP), 2007). Climate changes affect the dynamical structure and the chemical composition of the stratosphere in various ways through changes in the tropospheric wave forcing and through in situ changes in the radiative and chemical processes. The stratosphere might play a more significant and complex role in tropospheric dynamics and climate than previously thought. Recent studies have indicated that stratospheric dynamical perturbations, caused by internal variability or in-situ radiative forcings, may significantly influence the troposphere. Since ozone strongly interacts with the solar and terrestrial radiation, stratospheric ozone perturbations can directly influence tropospheric dynamics through changes to the radiative balance of the atmosphere (IPCC, 2001). Recent studies have shown that stratospheric ozone depletion in the Southern

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