Abstract
The 1:1 and 1:2 copper(II), nickel(II) and palladium(II) complexes of pyridine-2-2acetamide (abbreviation, paaH), α and βCuCl2(paaH), CuBr2 (paaH), CuCl2(paaH)2, CuBr2(paaH)2, Cu(ClO4)2(paaH)2, NiCl2(paaH)2 · 2H2O, PdCl2(paaH)2 and PdBr2(paaH)2, were prepared and their structure determined by magnetic moments, diffuse-reflactance and infrared spectra. The copper complexes have distorted octahedral or sqaure-planar structures, and the nickel complex an octahedral structure. In these complexes the ligand coordiantes to the metals through pyridine-N and amide-O atoms. The palladium complexes have square-planar structures with two unidentate paaH coordinating at the position through pyridine-N atoms.
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