Abstract

Abstract. The CHRONOS space mission concept provides time-resolved abundance for emissions and transport studies of the highly variable and highly uncertain air pollutants carbon monoxide and methane, with sub-hourly revisit rate at fine (∼ 4 km) horizontal spatial resolution across a North American domain. CHRONOS can provide complete synoptic air pollution maps (snapshots) of the continental domain with less than 10 min of observations. This rapid mapping enables visualization of air pollution transport simultaneously across the entire continent and enables a sentinel-like capability for monitoring evolving, or unanticipated, air pollution sources in multiple locations at the same time with high temporal resolution. CHRONOS uses a compact imaging gas filter correlation radiometer for these observations, with heritage from more than 17 years of scientific data and algorithm advances by the science teams for the Measurements of Pollution in the Troposphere (MOPITT) instrument on NASA's Terra spacecraft in low Earth orbit. To achieve continental-scale sub-hourly sampling, the CHRONOS mission would be conducted from geostationary orbit, with the instrument hosted on a communications or meteorological platform. CHRONOS observations would contribute to an integrated observing system for atmospheric composition using surface, suborbital and satellite data with atmospheric chemistry models, as defined by the Committee on Earth Observing Satellites. Addressing the U.S. National Academy's 2007 decadal survey direction to characterize diurnal changes in tropospheric composition, CHRONOS observations would find direct societal applications for air quality management and forecasting to protect public health.

Highlights

  • For the end of the current decade, geostationary Earth orbit (GEO) satellite missions for atmospheric composition are planned over North America, East Asia and Europe, with additional missions in formulation or proposed

  • From observing system simulation experiments (OSSEs), we have demonstrated that data assimilation of simulated CHRONOS multispectral observations of carbon monoxide (CO) significantly improves comparisons with the “true” surface CO values at EPA surface monitoring sites (Edwards et al, 2009)

  • It would deliver air pollutant measurements identified in the 2007 decadal survey GEO-CAPE mission (NRC, 2007) and address currently unmet science objectives described in the GEO-CAPE Science Traceability Matrix (Fishman et al, 2012)

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Summary

Introduction

For the end of the current decade, geostationary Earth orbit (GEO) satellite missions for atmospheric composition are planned over North America, East Asia and Europe, with additional missions in formulation or proposed. In addition to NASA’s TEMPO (Tropospheric Emissions: Monitoring Pollution) mission (Zoogman et al, 2017), the ESA/EUMETSAT (European Space Agency/European Organisation for the Exploitation of Meteorological Satellites) Sentinel-4 mission over Europe (GMES-GAS, 2009) and the Korean KARI (Korea Aerospace Research Institute) MP-GEOSAT/GEMS (Multi-Purpose Geostationary Satellite/Geostationary Environment Monitoring Spectrometer) mission over Asia (Lee et al, 2010) will provide data products for ozone (O3), nitrogen dioxide (NO2), sulfur dioxide (SO2), formaldehyde (HCHO) and aerosol optical depth (AOD) several times per day with smaller than 10 km × 10 km spatial footprints While these planned GEO measurements will provide new information. We show how CHRONOS would complement observations from other current and planned satellite instruments, and we conclude with a summary of CHRONOS features and advantages

CHRONOS sub-hourly synoptic measurements with high spatial resolution
The CHRONOS science objectives
CHRONOS measurements of CH4 and CO
GCFR concepts
Vacuum
Spectroscopy of CO and CH4 and the CHRONOS instrument signals
Measurement radiometric accuracy and precision
The CHRONOS instrument and operation
Multispectral CO measurements and vertical profile information
Retrieval sensitivity to near-surface CH4
Relationship of CHRONOS to current and future missions
Other satellite CO observations
Other satellite CH4 observations
Findings
Conclusions
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