Abstract

The effect of perturbations on the performance of an adiabatic reactor used for processing the exothermic catalytic oxidation of carbon monoxide has been investigated. Perturbations studied included, step changes in concentration and temperature, pulse changes in concentration, hysteresis effects and addition of CO 2 to the feed stream. Intraparticle temperatures were measured for some of these perturbations. The heterogeneous dispersion model was suitable for steady-state predictions but was not adequate for transient behaviour.

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