Abstract
The effect of fluctuations in the pulse duration of synchronously pumped modelocked pulse trains on excite and probe measurements is discussed. Relaxation times comparable with the pulse durations can be measured even when large pulse-to-pulse fluctuations in duration exist. The pump and probe pulse durations are assumed to be correlated. When the probe pulses are the second harmonic of the pump, or vice versa, the third harmonic must also be generated to permit deconvolution of experimental excite and probe data. When the pump and probe pulses have the same time dependence, the excite and probe curves consist of the desired response function convolved with the time-averaged second harmonic autocorrelation function which is easily measured. Deconvolution yields the relaxation time but fluctuations in pulse duration increase the root-mean-square voltage fluctuation at the output of the detector system and limit the accuracy with which the relaxation time can be calculated.
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