Abstract
We performed optical-pump terahertz-probe measurements of a Mott insulatorYTiO3 and a band semiconductor Si using a laser diode (1.47 eV) and a femtosecond-pulselaser (1.55 eV). Both samples possess long energy-relaxation times (1.5 ms forYTiO3 and 15 µs for Si); therefore, it is possible to extract terahertz complex conductivities of photoinducedcarriers under equilibrium. We observed highly contrasting behaviour—Drudeconductivity in Si and localized conductivity possibly obeying the Jonscher law inYTiO3. The carrier number at the highest carrier-concentration layer inYTiO3 is estimated to be 0.015 per Ti site. Anisotropic conductivity ofYTiO3 is determined. Our study indicates that localized carriers might play an important rolein the incipient formation of photoinduced metallic phases in Mott insulators.In addition, this study shows that the transfer-matrix method is effective forextracting an optical constant of a sample with a spatially inhomogeneous carrierdistribution.
Talk to us
Join us for a 30 min session where you can share your feedback and ask us any queries you have
Disclaimer: All third-party content on this website/platform is and will remain the property of their respective owners and is provided on "as is" basis without any warranties, express or implied. Use of third-party content does not indicate any affiliation, sponsorship with or endorsement by them. Any references to third-party content is to identify the corresponding services and shall be considered fair use under The CopyrightLaw.