Abstract
A novel strategy through a temperature-responsive dissolution and recrystallization process has successfully achieved 100% atomic utilization and easy recyclability of heterogeneous metal organic framework dimethylammonium zinc formate (DMZnF) catalysts for highly efficient dehydrogenation of DMF-H2O for hydrogen generation. DMZnF dissolves as a homogeneous catalyst at high reaction temperatures and then is recrystallized and recycled as a heterogeneous catalyst at low temperatures.
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