Abstract

AgGa1−xInxS2 with x=0.14±0.01 was found to be 90° phase-matchable for the second harmonic generation (SHG) of CO2 laser radiation at 10.591μm at 203°C. In addition, temperature-tuned 90° phase-matched difference frequency generation (DFG) at 4.02μm was demonstrated by mixing the idler output of a Nd:YAG third harmonic pumped β-BBO optical parametric oscillator and its fundamental source at 1.0642μm. The Sellmeier and thermo-optic dispersion formulas that reproduce well these experimental data are presented.

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