Abstract

Strain-engineering is used as a tool to alter electronic and magnetic properties like anisotropy energy. This study reports the different angle-dependent magnetoresistance properties of the strain-engineered La0.67Sr0.33MnO3 (LSMO) thin films, grown on LaAlO3, compared to their bulk analogs. Upon increasing temperature, a symmetry change from fourfold [cos(4θ)] to twofold [cos(2θ)] is observed in the angle-dependent resistance measurements. This systematic study with increasing temperature allows us to define three distinct temperature-dependent phases. The fourfold symmetric signal originates from magnetocrystalline anisotropy, whereas the twofold symmetric signal is believed to be the conventional anisotropic magnetoresistance. Our observations show that strain-engineering creates the possibility to manipulate the anisotropy, which, for example, can ultimately lead to observations of noncollinear quasi-particles like skyrmions in single layer thin films of LSMO.

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