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Abstract
With the rapid development of current electronic equipment, electromagnetic microwave absorption (EMA) materials with higher design requirements under special circumstances have attracted great attention. Herein, a flexible polyurethane composite foam assisted by coral‐like CNT@Fe3O4/graphene nanocomposites is fabricated by a facile solvothermal and moisture self‐foaming method. The composite foam with 15 wt% nanofillers exhibits an outstanding temperature cycle stability with gradually improved EMA performance at elevated temperature and excellent resilience stability with a tensile strength of 4.81 MPa. An enhanced minimum reflection loss (RLmin) of −59.44 dB at 10.38 GHz with a thickness of 2.28 mm is achieved, while the ultrawide absorption bandwidth of 6.09 GHz nearly covers the full X‐band. This benefits from interface impedance matching, dielectric and magnetic dual losses, and multiple reflections depending on the interior open microcellular structures. It is expected to become a promising thermally tunable microwave absorber in harsh environments.
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