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Abstract
Abstract The influence of elevated temperatures on the formation of 1:1 chloro complexes for Eu3+ and Am3+ are reported. Using a solvent extraction technique, stability constants for the equilibrium M(aq) 3++Cl(aq) – MCl(aq) 2+ have been measured in the temperature range of 25–75 °C. Modest increases in 1 are observed, and small positive enthalpies for these reactions are reported. These data are discussed in the context of previous reports for the trivalent lanthanide and actinide chloro systems.
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