Tailoring azimuthal optical force on lossy chiral particles in Bessel beams

Abstract

Based on the Mie scattering theory and Maxwell stress tensor method, we investigate the transverse optical force (TOF) acting on chiral particles illuminated by a zero-order Bessel beam. It is demonstrated that the particle chirality can induce an azimuthal optical force (AOF), resulting in orbital motion of particles around the optical beam axis. The AOF depends strongly on particle loss as well as the handedness of chirality, with its amplitude capable of changing by over an order of magnitude by particle's chiral loss. The other component of TOF, the radial optical force (ROF), is much less sensitive to the magnitude and handedness of the particle chirality as well as the loss when the chirality is small. Analytical result based on dipole approximation reveals that the AOF arises from the direct coupling of particle chirality to both the spin angular momentum (SAM) and optical vorticity (curl of Poynting vector), exhibiting a conversion of optical SAM of an incident beam to mechanical orbital angular momentum of an illuminated particle. Differently, the ROF originates from the transverse gradient force. In addition, particle chirality yields a negative contribution to the gradient force; thus the ROF can be attenuated and even reversed in direction when particle chirality is sufficiently large. These characteristics of TOF might find applications in chirality detection as well as sorting chiral particles of different handedness and separating them from conventional ones.