Abstract

The tunneling magnetoresistance (TMR) of granular films prepared by the co-deposition of well-defined ferromagnetic Co clusters and insulating inert-gas matrix atoms has been studied as function of matrix atoms (Kr, Xe), cluster volume fraction, temperature (4–40 K) and cluster size (4.2–5.2 nm). Tunneling samples with resistivities that differ by about five orders of magnitude have a TMR that is found to be independent of matrix and cluster volume fraction, i.e. is independent of both tunneling barrier height and width. All samples show a characteristic TMR( T)-dependence that can be explained by a model which takes into account that magnetic moments at the cluster surface are becoming misaligned with increasing temperature. The fraction of misaligned moments at a fixed temperature is increasing with decreasing clusters size.

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