Abstract
The first heterometal tetranuclear complex with alternating azido and phenoxo bridges, [Mn2Ni2(MeOSalen)2(μ1,1-N3)2(N3)2] (MeOSalenH2=bis(3-methoxy)salicylideneimine), was synthesized and structurally characterized by X-ray crystallography and spectroscopic methods. Magnetic studies suggest there is a ferromagnetic interaction between the μ1,1-azido-bridged Mn(II) ions with J=+2.11cm−1, while the Ni(II) ions are diamagnetic in the tetranuclear system.
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