Abstract
The new antiferromagnetic polymer [Cu(NH 2C 2H 4O)(NCS)]∞ has been prepared and shown by X-ray crystallography to contain a new polymeric linkage of pairs of copper(II) atoms linked alternately by two oxygen bridges and one weaker thiocyanate bridge. Electronic, ESR and IR spectra and temperature-variable magnetochemical data are described. [Ni(NH 2C 2H 4OH) 2(NCS) 2] is fully characterized by its magnetism, electronic and IR spectra and crystal structure as a centrosymmetric octahedral monomer with nitrogen-coordinated thiocyanates.
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