Abstract

Multicomponent oxides with pyrochlore structure (A2Zr2O6O’) containing up to 7 different cations with equiatomic amounts have been successfully synthesized, which broadens pyrochlore solid solutions to high entropy pyrochlore oxides. XRD and Raman results indicate that all compositions possessed single-phase pyrochlore structure and the HAADF-STEM images with corresponding EDS mapping demonstrate that all cations were randomly and homogeneously distributed. This new class of high-entropy pyrochlore oxides may open a new research direction in pyrochlore-based materials.

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