Abstract
Hydrogenation of the alkylidyne bridged dimer [(cb) 2Ta(μ-CSiMe 3) 2Ta(cb) 2] (cbH = 9H-carbazole) in the presence of PMe 2Ph leads to the green hexahydride compound [(cb)(PMe 2Ph) 2(H)Ta(μ-H) 4Ta(H)(PMe 2Ph) 2(cb)] which contains a TaTa distance of 2.5359(4) Å and TaN (carbazole) distance of 2.184(4) Å.
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