Abstract
AbstractA crystallographically characterized three‐coordinate, formally 14 electron PtII complex 1 featuring terminal amido ligation is reported. Computational analysis revealed relatively weak π donation from the amide lone pair to platinum and supports a 14‐electron assignment for 1. Stoichiometric reactivity studies confirmed the viability of net OH and CH addition across, as well as isonitrile insertion into, the terminal platinum–amido linkage of 1.
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