Abstract
Conjugated benzenoid aromatics with large inner cavities and alkyl side chains self-associate to produce dimers in solution and fibrous materials in the solid state. The self-association is enthalpically and entropically driven. The compound forms a 1:3 charge-transfer (CT) complex with 2,4,7-trinitrofluorenone (TNF) with a microball structure, where a nano-sized branched structure forms first at the growth points, followed by production of the microball with a dendritic interior.
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