Abstract

Abstract. The exploration of aerosol retrieval synergies from diverse combinations of ground-based passive Sun-photometric measurements with collocated active lidar ground-based and radiosonde observations using versatile Generalized Retrieval of Atmosphere and Surface Properties (GRASP) algorithm is presented. Several potentially fruitful aspects of observation synergy were considered. First, a set of passive and active ground-based observations collected during both day- and nighttime was inverted simultaneously under the assumption of temporal continuity of aerosol properties. Such an approach explores the complementarity of the information in different observations and results in a robust and consistent processing of all observations. For example, the interpretation of the nighttime active observations usually suffers from the lack of information about aerosol particles sizes, shapes and complex refractive index. In the realized synergy retrievals, the information propagating from the nearby Sun-photometric observations provides sufficient constraints for reliable interpretation of both day- and nighttime lidar observations. Second, the synergetic processing of such complementary observations with enhanced information content allows for optimizing the aerosol model used in the retrieval. Specifically, the external mixture of several aerosol components with predetermined sizes, shapes and composition has been identified as an efficient approach for achieving reliable retrieval of aerosol properties in several situations. This approach allows for achieving consistent and accurate aerosol retrievals from processing stand-alone advanced lidar observations with reduced information content about aerosol columnar properties. Third, the potential of synergy processing of the ground-based Sun-photometric and lidar observations, with the in situ backscatter sonde measurements was explored using the data from KAUST.15 and KAUST.16 field campaigns held at King Abdullah University of Science and Technology (KAUST) in the August of 2015 and 2016. The inclusion of radiosonde data has been demonstrated to provide significant additional constraints to validate and improve the accuracy and scope of aerosol profiling. The results of all retrieval setups used for processing both synergy and stand-alone observation data sets are discussed and intercompared.

Highlights

  • Ground-based remote sensing is widely recognized as a valuable source of information about the details of the optical properties of ambient atmospheric aerosols (e.g. IPCC, 2013)

  • Lopatin et al.: Synergy processing of diverse ground-based remote sensing using the Generalized Retrieval of Atmosphere and Surface Properties (GRASP) algorithm clude the spectral observations of the direct-Sun radiation as well as the multi-angular polarimetric spectral observations of diffuse Sun radiation transmitted through the atmosphere

  • Recently proposed Lidar and Radiometer Inversion Code (LiRIC) (Chaikovsky et al, 2016) and Generalized Aerosol Retrieval form Radiometer and Lidar Combination/Generalized Retrieval of Atmosphere and Surface Properties (GARRLiC/GRASP) (Lopatin et al, 2013) algorithms use the joint data from a multi-wavelength lidar and an Aerosol Robotic Network (AERONET) Sun–skyscanning radiometer to derive vertical profiles of fine and coarse aerosol components as well as extra parameters of the column-integrated properties of aerosols

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Summary

Introduction

Ground-based remote sensing is widely recognized as a valuable source of information about the details of the optical properties of ambient atmospheric aerosols (e.g. IPCC, 2013). As shown in numerous studies, the main aerosol properties including aerosol size distribution, complex refractive index and information about particle shape can be successfully retrieved from the spectral direct-Sun and sky-scanning ground-based observations of atmospheric radiation This paper demonstrates the potential of synergy processing of the ground-based remote sensing observations together with advanced lidar or backscatter sonde data (that can be considered as a certain in situ analogue of lidar backscattering measurements). 3. GRASP is a highly versatile algorithm that is developed based on very general principles of numerical inversion and atmospheric radiation modelling which allows utilization of the same algorithm in diverse applications, including processing of passive and active remote sensing observations from the ground, space and aircraft including in situ measurements. Other details on GRASP operational principles and application to different observation types could be found in Dubovik et al (2000, 2006, 2011) and Lopatin et al (2013)

Modelling of aerosol optical properties
Vertically resolved measurements in GRASP: lidars and airborne instruments
Numerical inversion and retrieval constraints
Multi-instrumental retrievals
Stand-alone instrumental retrievals
Stand-alone COBALD retrievals
Stand-alone LILAS retrievals
Findings
Conclusions
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