Abstract
Helium (^{4}He) nanodroplets provide a unique environment to observe the microscopic origins of superfluidity. The search for another superfluid substance has been an ongoing quest in the field of quantum fluids. Nearly two decades ago, experiments on doped parahydrogen (p-H_{2}) clusters embedded in ^{4}He droplets displayed anomalous spectroscopic signatures that were interpreted as a sign of the superfluidity of p-H_{2} [S. Grebenev etal., Science 289, 1532 (2000)SCIEAS0036-807510.1126/science.289.5484.1532]. Here, we observe, using first-principles quantum MonteCarlo simulations, a phase separation between a symmetric and localized p-H_{2} core and ^{4}He shells. The p-H_{2} core has minimal superfluid response. These findings are consistent with the recorded spectra but not with their original interpretation, and lead us to conclude that doped p-H_{2} clusters form a nonsuperfluid core in ^{4}He droplets.
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