Abstract

Sr2IrO4 has been shown to exhibit a novel Jeff = 1/2 Mott spin–orbit insulating state with antiferromagnetic ordering. In the present investigation, the effects of Pr substitution at Sr-site on structural, magnetic and electrical properties are studied in Sr2IrO4. Pr-doped samples still retain the insulating behavior, but with the increase of Pr doping concentration, the resistivity decreases. The magnetic properties show that long-range antiferromagnetic order is collapsed when the Pr doping content increases up to 20%, which may results from a competition between the AFM (Ir 5d electrons) and ferromagnetic (Pr 4 f electrons) coupling. In addition, Pr doping induces a spin glasslike state at low temperatures.

Talk to us

Join us for a 30 min session where you can share your feedback and ask us any queries you have

Schedule a call

Disclaimer: All third-party content on this website/platform is and will remain the property of their respective owners and is provided on "as is" basis without any warranties, express or implied. Use of third-party content does not indicate any affiliation, sponsorship with or endorsement by them. Any references to third-party content is to identify the corresponding services and shall be considered fair use under The CopyrightLaw.