Superferromagnetism and coercivity in Co-Al2O3 granular films with perpendicular anisotropy

Abstract

Magnetic properties of nano-granular Co0.55–(Al2O3)0.45 films have been studied by vibrating sample magnetometry, ferromagnetic resonance, and magnetic force microscopy (MFM). The films possess a growth-induced perpendicular anisotropy related to the shape anisotropy of the granules. Being unpercolated physically, the films demonstrated a clear magnetic percolation behavior in the temperature dependence of the coercivity and MFM scans. The temperature dependence of the coercivity measured along the easy magnetization axis of the granules indicates the presence of a collective long-range magnetic state sustained by a ferromagnetic interparticle interaction. This interaction is supposed to form a homogeneously magnetized superferromagnetic state, however, the perpendicular anisotropy and the competition between the dipole-dipole and ferromagnetic interactions lead to the emergence of an inhomogeneous labyrinth-like magnetic stripe-domain structure with the averaged domain width being about two orders of magnitude larger than the averaged granule size. The temperature evolution of the spontaneous magnetization inside the stripe domains has been measured by the MFM up to the temperature of superferromagnetic ordering (420 K). The formerly developed mean-field-based model of the coercivity of an interacted ensemble has been tested and found to yield adequate quantitative predictions.